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Enhanced reductive degradation of carbon tetrachloride by carbon dioxide radical anion-based sodium percarbonate

Wenchao Jiang, Ping Tang, Shuguang Lu, Xiang Zhang, Zhaofu Qiu, Qian Sui

《环境科学与工程前沿（英文）》 2018年 第12卷 第2期 doi: 10.1007/s11783-017-0987-6

摘要： The performance of sodium percarbonate (SPC) activated with ferrous ion (Fe(II)) with the addition of formic acid (FA) to stimulate the degradation of carbon tetrachloride (CT) was investigated. Results showed that CT could be entirely reduced within 15 min in the system at a variety of SPC/Fe(II)/FA/CT molar ratios in experimental level. Scavenging tests indicated that carbon dioxide radical anion (CO2· ) was the dominant reactive oxygen species responsible for CT degradation. CT degradation rate, to a large extent, increased with increasing dosages of chemical agents and the optimal molar ratio of SPC/Fe(II)/FA/CT was set as 60/60/60/1. The initial concentration of CT can hardly affect the CT removal, while CT degradation was favorable in the pH range of 3.0–9.0, but apparently inhibited at pH 12. Cl and HCO of high concentration showed negative impact on CT removal. Cl released from CT was detected and the results confirmed nearly complete mineralization of CT. CT degradation was proposed by reductive C-Cl bond splitting. This study demonstrated that SPC activated with Fe(II) with the addition of FA may be promising technique for CT remediation in contaminated groundwater.

关键词： Carbon tetrachloride     Sodium percarbonate     Formic acid     Reductive radicals     Groundwater    

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Degradation of carbon tetrachloride in thermally activated persulfate system in the presence of formic

Minhui XU,Xiaogang GU,Shuguang LU,Zhouwei MIAO,Xueke ZANG,Xiaoliang WU,Zhaofu QIU,Qian SUI

《环境科学与工程前沿（英文）》 2016年 第10卷 第3期   页码 438-446 doi: 10.1007/s11783-015-0798-6

摘要： The thermally activated persulfate (PS) degradation of carbon tetrachloride (CT) in the presence of formic acid (FA) was investigated. The results indicated that CT degradation followed a zero order kinetic model, and was responsible for the degradation of CT confirmed by radical scavenger tests. CT degradation rate increased with increasing PS or FA dosage, and the initial CT had no effect on CT degradation rate. However, the initial solution pH had effect on the degradation of CT, and the best CT degradation occurred at initial pH 6. Cl had a negative effect on CT degradation, and high concentration of Cl displayed much strong inhibition. Ten mmol·L promoted CT degradation, while 100 mmol·L inhibited the degradation of CT, but promoted CT degradation in the presence of FA. The measured Cl concentration released into solution along with CT degradation was 75.8% of the total theoretical dechlorination yield, but no chlorinated intermediates were detected. The split of C-Cl was proposed as the possible reaction pathways in CT degradation. In conclusion, this study strongly demonstrated that the thermally activated PS system in the presence of FA is a promising technique in in situ chemical oxidation (ISCO) remediation for CT contaminated site.

关键词： persulfate     carbon tetrachloride     thermal activation     formic acid     carbon dioxide radical anion    

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Rdh13 deficiency weakens carbon tetrachloride-induced liver injury by regulating Spot14 and Cyp2e1 expression

Xiaofang Cui, Benting Ma, Yan Wang, Yan Chen, Chunling Shen, Ying Kuang, Jian Fei, Lungen Lu, Zhugang Wang

《医学前沿（英文）》 2019年 第13卷 第1期   页码 104-111 doi: 10.1007/s11684-017-0568-x

摘要： Mitochondrion-localized retinol dehydrogenase 13 (Rdh13) is a short-chain dehydrogenase/reductase involved in vitamin A metabolism in both humans and mice. We previously generated knockout mice and showed that Rdh13 deficiency causes severe acute retinal light damage. In this study, considering that Rdh13 is highly expressed in mouse liver, we further evaluated the potential effect of Rdh13 on liver injury induced by carbon tetrachloride (CCl ). Although Rdh13 deficiency showed no significant effect on liver histology and physiological functions under regular culture, the mice displayed an attenuated response to CCl -induced liver injury. Their livers also exhibited less histological changes and contained lower levels of liver-related metabolism enzymes compared with the livers of wild-type (WT) mice. Furthermore, the mice had Rdh13 deficiency and thus their liver cells were protected from apoptosis, and the quantity of their proliferative cells became lower than that in WT after CCl exposure. The ablation of gene decreased the expression levels of thyroid hormone-inducible nuclear protein 14 (Spot14) and cytochrome P450 (Cyp2e1) in the liver, especially after CCl treatment for 48 h. These data suggested that the alleviated liver damage induced by CCl in mice was caused by Cyp2e1 enzymes, which promoted reductive CCl metabolism by altering the status of thyroxine metabolism. This result further implicated Rdh13 as a potential drug target in preventing chemically induced liver injury.

关键词： retinol dehydrogenase 13     carbon tetrachloride     acute liver injury     Cyp2e1     Spot14    

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Enhanced carbon tetrachloride degradation by hydroxylamine in ferrous ion activated calcium peroxide

Wenchao Jiang, Ping Tang, Zhen Liu, Huan He, Qian Sui, Shuguang Lyu

《环境科学与工程前沿（英文）》 2020年 第14卷 第2期 doi: 10.1007/s11783-019-1197-1

摘要： Complete CT degradation was achieved by employing HA to CP/Fe(II)/FA process. Quantitative detection of Fe(II) regeneration and HO• production was investigated. Benzoic acid outcompeted FA for the reaction with HO•. CO2•− was the dominant reductive radical for CT removal. Effects of solution matrix on CT removal were conducted. Hydroxyl radicals (HO•) show low reactivity with perchlorinated hydrocarbons, such as carbon tetrachloride (CT), in conventional Fenton reactions, therefore, the generation of reductive radicals has attracted increasing attention. This study investigated the enhancement of CT degradation by the synergistic effects of hydroxylamine (HA) and formic acid (FA) (initial [CT] = 0.13 mmol/L) in a Fe(II) activated calcium peroxide (CP) Fenton process. CT degradation increased from 56.6% to 99.9% with the addition of 0.78 mmol/L HA to the CP/Fe(II)/FA/CT process in a molar ratio of 12/6/12/1. The results also showed that the presence of HA enhanced the regeneration of Fe(II) from Fe(III), and the production of HO• increased one-fold when employing benzoic acid as the HO• probe. Additionally, FA slightly improves the production of HO•. A study of the mechanism confirmed that the carbon dioxide radical (CO2•−), a strong reductant generated by the reaction between FA and HO•, was the dominant radical responsible for CT degradation. Almost complete CT dechlorination was achieved in the process. The presence of humic acid and chloride ion slightly decreased CT removal, while high doses of bicarbonate and high pH inhibited CT degradation. This study helps us to better understand the synergistic roles of FA and HA for HO• and CO2•− generation and the removal of perchlorinated hydrocarbons in modified Fenton systems.

关键词： Calcium peroxide     Hydroxylamine     Modified Fenton     Reactive oxygen species     Perchlorinated hydrocarbon    

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AGRICULTURAL GREEN DEVELOPMENT TO ACHIEVE FOOD SECURITY AND CARBON REDUCTION IN THE CONTEXT OF CHINA’S DUAL CARBON GOALS

《农业科学与工程前沿（英文）》 2023年 第10卷 第2期   页码 262-267 doi: 10.15302/J-FASE-2023496

摘要：

● To achieve food security, Chinese agriculture– food system could not achieve C neutrality.

关键词： agriculture     carbon neutrality     carbon peak     food security     carbon mitigation strategies    

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Research on low carbon management using a scientific classification method

Shanna QI, Meiting JU, Meng DUAN, Wei XING

《环境科学与工程前沿（英文）》 2012年 第6卷 第4期   页码 524-530 doi: 10.1007/s11783-011-0333-3

摘要： This research is aimed at the rapid development of a low-carbon economy, in which we propose the classification and application of relevant management measures to affect the development of environmental management ideas and measures of the low-carbon economy, which we called as low carbon management measures. According to scientific analysis of the low-carbon economy, we can divide low-carbon management measures into three parts: measures for reduction of carbon sources, carbon flow planning, and increase of carbon sinks. Furthermore, we list the advantages that China can utilize to develop its own low-carbon management measures. In the end, necessary adjustments to environmental management measures in China can be made according to this scientific classification.

关键词： low-carbon economy     low carbon management     carbon source     carbon flow     carbon sink    

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Thoughts on strategies and paths to achieve carbon peaking and carbon neutrality in China

《能源前沿（英文）》 2023年 第17卷 第3期   页码 324-331 doi: 10.1007/s11708-023-0883-7

摘要： First, a brief introduction is made to the four basic judgments and understandings of the goals of “carbon peaking and carbon neutrality.” Then, an in-depth elaboration is provided on the eight major strategies for achieving the goals of “carbon peaking and carbon neutrality,” including conservation and efficiency priority, energy security, non-fossil energy substitution, re-electrification, resource recycling, carbon sequestration, digitalization and cooperation between countries. Next, eight major implementation paths for achieving the goals of “carbon peaking and carbon neutrality” are discussed in detail, including industrial restructuring; building a clean, low-carbon, safe and efficient energy system, and renewing the understanding of China’s energy resource endowment; accelerating the construction of a new-type power system with a gradually growing proportion of new energy, and realizing the “possible triangle” of high-quality energy system development; utilizing electrification and deep decarbonization technologies to promote the orderly peaking and gradual neutralization of carbon emissions in the industrial sector; promoting the low-carbon transition of transportation vehicles to achieve carbon peaking and carbon neutrality in the transportation sector; focusing on breaking through key green building technologies to achieve zero carbon emissions from building electricity and heat; providing a strong technical support for carbon removal to achieve carbon neutrality; accelerating the construction of the integrated planning and assessment mechanism for pollution and carbon reduction, establishing a sound strategy, planning, policy and action system, and optimizing the carbon trading system. Afterwards, it is particularly pointed out that the realization of the goals of “carbon peaking and carbon neutrality” cannot be separated from the support of sci-tech innovation. Finally, it is stressed that carbon neutrality is not the end, but an important milestone. If viewed from the perspective of future energy, the significance and historical status of the goals of “carbon peaking and carbon neutrality” will be more understandable.

关键词： carbon peaking and carbon neutrality     strategy     implementation path     important sci-tech innovation implementation path    

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HIGHLIGHTS OF THE SPECIAL ISSUE “CARBON NEUTRALITY AND A LOW CARBON ECONOMY FOR AGRICULTURE”

《农业科学与工程前沿（英文）》 2023年 第10卷 第2期   页码 153-154 doi: 10.15302/J-FASE-2023497

摘要： HIGHLIGHTS OF THE SPECIAL ISSUE “CARBON NEUTRALITY AND A LOW CARBON ECONOMY FOR AGRICULTURE”

关键词： CARBON     ISSUE     NEUTRALITY     HIGHLIGHTS     AGRICULTURE    

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LIVESTOCK AND POULTRY MANURE MANAGEMENT FROM THE PERSPECTIVE OF CARBON NEUTRALITY IN CHINA

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 341-362 doi: 10.15302/J-FASE-2023509

摘要：

● Carbon reduction potential of manure treatment technologies was summarized.

关键词： valorization of animal manure     manure management     carbon emission     carbon footprint     methodology     carbon trading    

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Correlation between carbon emissions and energy structure –Reliability analysis of low carbon target

Ben HUA

《能源前沿（英文）》 2011年 第5卷 第2期   页码 214-220 doi: 10.1007/s11708-010-0133-7

摘要： The influence of energy intensity on carbon intensity depends upon the fraction of energy mixes with high carbon emissions in the total energy mixes . The correlation of with a variety of primary energy mix fractions and technology advances such as CCS and CCHP is analyzed and deduced. Taking the long-term carbon reduction target in 2050 settled upon by the Copenhagen Agreement and the mid-term target suggested by the “450 Scenes Program” of the International Energy Agency (IEA) as constraints, the new pattern of the energy transition of the world in 2020, 2030, and 2050 are estimated and figured out. The peak value of energy consumption will lag behind the peak value of carbon emissions; the world energy structure shifting point will be in 2020–2025. Estimates show that China’s mid-2020 and long-term targets of energy-saving and emission reduction announced by the Chinese government might be achieved.

关键词： correlation     carbon emissions     energy consumption     high carbon emissions energy mix     target of emission reduction     reliability    

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A global carbon market?

Michael G. POLLITT

《工程管理前沿（英文）》 2019年 第6卷 第1期   页码 5-18 doi: 10.1007/s42524-019-0011-x

摘要：

This paper explores the prospects for a global carbon market as the centerpiece of any serious attempt to reach the ambitious goal for greenhouse gas (GHG) reductions set by climate scientists. My aim is to clarify the extent to which we know what policy might best support global decarbonisation. We begin by discussing what we might mean by a global carbon market and its theoretical properties. We then go on to discuss the EU Emissions Trading System experience and the recent experience with the Australian carbon tax. Next, we assess recent carbon market initiatives in the US and in China. My argument is that while establishing the amount of emissions required and dividing it up acceptably between countries requires an enormous scientific and international negotiations effort, the economic instruments to deliver the agreed targets are readily at hand.

关键词： carbon market     carbon tax     EU ETS    

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Insights into carbon-based materials for catalytic dehydrogenation of low-carbon alkanes and ethylbenzene

《化学科学与工程前沿（英文）》 2023年 第17卷 第11期   页码 1623-1648 doi: 10.1007/s11705-023-2328-6

摘要： Direct dehydrogenation with high selectivity and oxidative dehydrogenation with low thermal limit has been regarded as promising methods to solve the increasing demands of light olefins and styrene. Metal-based catalysts have shown remarkable performance for these reactions, such as Pt, CrOx, Co, ZrOx, Zn and V. Compared with metal-based catalysts, carbon materials with stable structure, rich pore texture and large surface area, are ideal platforms as the catalysts and the supports for dehydrogenation reactions. In this review, carbon materials applied in direct dehydrogenation and oxidative dehydrogenation reactions including ordered mesoporous carbon, carbon nanodiamond, carbon nanotubes, graphene and activated carbon, are summarized. A general introduction to the dehydrogenation mechanism and active sites of carbon catalysts is briefly presented to provide a deep understanding of the carbon-based materials used in dehydrogenation reactions. The unique structure of each carbon material is presented, and the diversified synthesis methods of carbon catalysts are clarified. The approaches for promoting the catalytic activity of carbon catalysts are elaborated with respect to preparation method optimization, suitable structure design and heteroatom doping. The regeneration mechanism of carbon-based catalysts is discussed for providing guidance on catalytic performance enhancement. In addition, carbon materials as the support of metal-based catalysts contribute to exploiting the excellent catalytic performance of catalysts due to superior structural characteristics. In the end, the challenges in current research and strategies for future improvements are proposed.

关键词： carbon materials     dehydrogenation     active sites     mechanism     catalytic performance     support    

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VALORIZATION OF LIVESTOCK WASTE AND CARBON NEUTRALITY

《农业科学与工程前沿（英文）》 2023年 第10卷 第3期   页码 333-340 doi: 10.15302/J-FASE-2023513

摘要： VALORIZATION OF LIVESTOCK WASTE AND CARBON NEUTRALITY

关键词： WASTE     CARBON     VALORIZATION     NEUTRALITY    

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Hierarchically porous zeolites synthesized with carbon materials as templates

《化学科学与工程前沿（英文）》 2021年 第15卷 第6期   页码 1444-1461 doi: 10.1007/s11705-021-2090-6

摘要： Hierarchically porous zeolites are promising candidates in catalytic conversion of relatively bulky molecules, and their syntheses have attracted significant attention. From both industrial and scientific perspectives, different carbon materials have been widely employed as hard templates for the preparation of hierarchically porous zeolites during the past two decades. In this review, the progress in synthetic strategies using carbon materials as templates is comprehensively summarized. Depending on the affinity between the carbon templates and zeolite precursors, the substantial strategies for synthesizing hierarchical zeolites are introduced in direct templates and indirect templates. Direct templates methods, by which the carbon materials are directly mixed with precursors gel as hard templates, are first reviewed. Then, we discuss the indirect templates method (crystallization of carbon-silica composites), by which the carbon is produced by in situ pyrolysis of organic-inorganic precursors. In addition, the technique of encapsulating metal species into zeolites crystals with the assistance of carbon templates is also discussed. In the conclusion part, the factors affecting the synthesis of carbon-templated hierarchically porous zeolites are remarked. This review is expected to attract interest in the synthesis strategies of hierarchically porous zeolites, especially cost-effective and large-scale production methodologies, which are essential to the industrial application of hierarchical zeolites.

关键词： hierarchical zeolites     carbon materials     direct templates     indirect templates     carbon-silica composites    

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SOIL CARBON CHECK: A TOOL FOR MONITORING AND GUIDING SOIL CARBON SEQUESTRATION IN FARMER FIELDS

《农业科学与工程前沿（英文）》 2023年 第10卷 第2期   页码 248-261 doi: 10.15302/J-FASE-2023499

摘要：

● Establishment of a rapid tool for monitoring soil carbon sequestration in farmer fields.

关键词： 4 per 1000 initiative     carbon sequestration     climate action     farmer fields     SDG13     soil organic carbon     soil testing    

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标题 作者 时间 类型 操作

Enhanced reductive degradation of carbon tetrachloride by carbon dioxide radical anion-based sodium percarbonate

Wenchao Jiang, Ping Tang, Shuguang Lu, Xiang Zhang, Zhaofu Qiu, Qian Sui

期刊论文

Degradation of carbon tetrachloride in thermally activated persulfate system in the presence of formic

Minhui XU,Xiaogang GU,Shuguang LU,Zhouwei MIAO,Xueke ZANG,Xiaoliang WU,Zhaofu QIU,Qian SUI

期刊论文

Rdh13 deficiency weakens carbon tetrachloride-induced liver injury by regulating Spot14 and Cyp2e1 expression

Xiaofang Cui, Benting Ma, Yan Wang, Yan Chen, Chunling Shen, Ying Kuang, Jian Fei, Lungen Lu, Zhugang Wang

期刊论文

Enhanced carbon tetrachloride degradation by hydroxylamine in ferrous ion activated calcium peroxide

Wenchao Jiang, Ping Tang, Zhen Liu, Huan He, Qian Sui, Shuguang Lyu

期刊论文

AGRICULTURAL GREEN DEVELOPMENT TO ACHIEVE FOOD SECURITY AND CARBON REDUCTION IN THE CONTEXT OF CHINA’S DUAL CARBON GOALS

期刊论文

Research on low carbon management using a scientific classification method

Shanna QI, Meiting JU, Meng DUAN, Wei XING

期刊论文

Thoughts on strategies and paths to achieve carbon peaking and carbon neutrality in China

期刊论文

HIGHLIGHTS OF THE SPECIAL ISSUE “CARBON NEUTRALITY AND A LOW CARBON ECONOMY FOR AGRICULTURE”

期刊论文

LIVESTOCK AND POULTRY MANURE MANAGEMENT FROM THE PERSPECTIVE OF CARBON NEUTRALITY IN CHINA

期刊论文

Correlation between carbon emissions and energy structure –Reliability analysis of low carbon target

Ben HUA

期刊论文

A global carbon market?

Michael G. POLLITT

期刊论文

Insights into carbon-based materials for catalytic dehydrogenation of low-carbon alkanes and ethylbenzene

期刊论文

VALORIZATION OF LIVESTOCK WASTE AND CARBON NEUTRALITY

期刊论文

Hierarchically porous zeolites synthesized with carbon materials as templates

期刊论文

SOIL CARBON CHECK: A TOOL FOR MONITORING AND GUIDING SOIL CARBON SEQUESTRATION IN FARMER FIELDS

期刊论文